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1.
INTRODUCTION
2.
EXPERIMENTAL METHODOLOGY
40
Irradiation Cross
Time
Section
(hours)
(barns)
Half-Life Foil
Nominal
(hours)
Mass (g) Thickness
(mm)
Au
197 Au(n.)198 Au
99,57
64,56
0,02727 0,0254
Au*
197 Au(n,)198 Au
15630**
64,56
0,02744 0,0254
Sc
45 Sc(n,)46 Sc
27,21
2011,92
0,05400 0,127
Sc**
45 Sc(n,)46 Sc
11,18**
2011,92
0,05218 0,127
2,72
56,4
0,12265 0,1016
56,4
U*
277,4**
Ti*
48 Ti(n,p)48 Sc
2,59.104 44,00
Ti
47 Ti(n,p)47 Sc
1,76.102 80,16
0,14463 0,254
Ti*
47 Ti(n,p)47 Sc
1,76.102 80,16
0,14050 0,254
Ni
58 Ni(n,p)58 Co
62,4.103 1728
0,28500 0,254
Ni*
58 Ni(n,p)58 Co
62,4.103 1728
0,28500 0,254
Mg
24 Mg(n,p)24 Na
1,47.103 15,06
0,03152 0,127
Mg*
24 Mg(n,p)24 Na
1,47.103 15,06
0,03152 0,127
In
115 In(n,n)115m In
183.103
4,50
0,12200 0,127
In*
115 In(n,n)115m In
183.103
4,50
Al*
27 Al(n,)24 Na
6,86.104 15,06
0,11103 0,1016
0,14170 0,254
0,12200 0,127
0,00446 0,127
2.1.
Irradiation Conditions
3.
2.2.
Gamma Spectrometry
The net counts (C) for each gamma energy peak in the
gamma foil spectrometry make possible to estimate the absolute activity if known its global efficiency (). The gamma
peak is emitted with an emission probability (I).Thus known
41
Daughter Gamma
Saturated Measured Activity***
Nuclide Photopeak (DPS/Nucleus)
(keV)**
Calculated Activity
by SANDBP Code
(DPS/Nucleus)
Au
198 Au
411,8
2,868.1013 6,46%
2,573.1013
Au*
198 Au
411,8
1,964.1013
6,46%
1,853.1013
Sc
46 Sc
889,20
1,945.1014 3,24%
2,007.1014
Sc*
46 Sc
889,2
1,470.1015
1,38%
1,506.1015
239 Np
277,6
2,670.1014 7,67%
3,274.1014
U*
239 Np
277,6
2,724.1014
7,67%
3,020.1014
Ti*
48 Sc
983,5
4,161.1019 4,76%
4,100.1019
Ti
47 Sc
159,4
3,994.1017
12,9%
3,369.1017
Ti*
47 Sc
159,4
3,307.1017 12,9%
3,305.1017
Ni
58 Co
810,8
2,011.1016
3,92%
1,948.1016
Ni*
58 Co
810,8
1,971.1016 3,92%
1,933.1016
Mg
24 Na
1368,5
3,311.1016
5,12%
2,299.1018
Mg*
24 Na
1368,5
3,570.1016 3,09%
2,272.1018
In
115m In
336,2
2,277.1018 3,36%
3,642.1016
In*
115m In
336,2
2,077.1018
7,26%
3,620.1016
Al* 24 Na
1368,5
1,251.1018 8,04%
Standard Deviation of Measured Activity
1,094.1018
9,90%
* cadmium covered; ** net peak counts during the gamma spectrometry; *** Corrected to
self-shielding effect.
C..e(.tw )
CF
I.. 1 e.tc 1 e.ti
(3.1)
A .W
m.NA . fiso
(3.2)
FIG. 2: Neutron Spectrum at the Central Position of the IPEN/MB01 Reactor Core obtained by SANDBP Code (3 iterations) to 51
energy points/5/ .
42
4.
FINAL COMMENTS
5,1312.109
1,6092.108
< 0,20.106
8,3502.108
4,9141.107
< 0,56.106
9,8087.108
4,9744.107
> 0,1
2,4771.109
6,7100.107
>0,4
2,0110.109
6,1730.107
>0,5
1,9040.109
6,3896.107
>1,0
1,3899.109
4,4776.107
The best neutron spectrum adjusted at experimental values (saturated activity per target nucleus) and initial guess
spectrum calculated by transport theory (Hammer-technion
cellular code) showed a 9,91% standard deviation between
experimental values (saturated activity per target nucleus)
and those obtained by SANDBP Code to adjusted neutron
spectrum. When are compared the integral neutron flux obtained by SANDBP Code with calculated values obtained
by CITATION/6/ code (Diffusion Theory using HammerTechnion data input to Cross Section in collapsed Groups
) at central position of the core is possible to see that there
are a good agreement between both methodologies. This can
be sawn in the Table 4. The calculated value is sub estimated
about 5% .The same way when are compared the shape of
the initial neutron spectrum (Hammer-Technion) and that obtained by SANDBP Code after 3 iterations how can be sawn
at Figure 2. For future works will very interesting to change
the initial guess neutron spectrum to make an analysis of the
sensitivity in the final neutron spectrum results. The same
way would be interesting to use more activation foils of different materials to cover specially the intermediate region of
the neutron spectrum.
Brazilian
Journal
of Physics,Neutron
vol. 39, Flux
no. 1,atMarch,
2009Position of the
TABLE
4: Integral
Central
IPEN/MB-01 (Standard Configuration of 28 26 fuel rods.
4,87.109
C/E
(0,95 0,06*)
FIG. 3: Comparative Graphics between Initial Guess Spectrum calculated by Hammer-Technion Cellular Code and that obtained by
Experimental Values Using the SANDBP Code. The Spectrum is
presented in Lethargy Units.
The neutron spectrum is a very important reactor physics parameter. Its understanding to take possible the estimation of
nuclear reaction rates and the neutron flux values. These results are important and may be used to check and validate
reactor physics codes and different nuclear data libraries.
43
Aiken, S.C., Du Pont de Nemours, Savannah River Laboratory,
1967.
[5] F.P.G. Martins, Medida do Espectro de Energia dos Nutrons no
Ncleo do Reator IPEN/MB-01. Dissertao de Mestrado, IPEN,
2006.
[6] T.B. Fowler et al. Citation Code, ORNL-TM-2496 Report, V r.
2, Suppl. 3, July, 1972.