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Junping Zhang
Research Associate Developing Vertical GasLiquid
Norman Epstein
Professor Emeritus
Upflow Using a Conductivity
Probe
John R. Grace
Professor Experiments were carried out in an 82.6-mm-dia column with a perforated distributor
plate. Conductivity probes on the axis of the column were used to measure local bubble
Department of Chemical Engineering, properties in the developing flow region for superficial air velocities from 0.0018 to 6.8
The University of British Columbia, m/s and superficial water velocities from 0 to 0.4 m/s, corresponding to the discrete
2216 Main Mall, bubble, dispersed bubble, coalesced bubble, slug, churn, bridging, and annular flow re-
Vancouver, BC, Canada V6T 1Z4 gimes. Bubble frequency increased linearly with gas velocity in the discrete and dispersed
bubble regimes. Bubble frequency also increased with gas velocity in the slug flow re-
gime, but decreased in the churn and bridging regimes. Bubble chord length and its
Kokseng Lim distribution were smaller and narrower in the dispersed than in the discrete bubble
Research Scientist, regime. Both the average and standard deviation of the bubble chord length increased
Fluidization Research Lab, with gas velocity in the discrete, dispersed, and churn flow regimes. However, the average
CSIRO Minerals, bubble chord length did not change significantly in the slug flow regime due to the high
Box 312, Clayton South, population of small bubbles in the liquid plugs separating Taylor bubbles. The bubble
Victoria, 3169 Australia travel length, defined as the product of local gas holdup and local bubble velocity divided
by local bubble/void frequency, is used to correlate bubble characteristics and to char-
acterize the flow regimes. S0098-22020000101-2
138 Vol. 122, MARCH 2000 Copyright 2000 by ASME Transactions of the ASME
location and the minimum or maximum of the signal voltage,
depending on the skewness of the signal. Several different thresh-
olds were set to check the effect of the threshold on the experi-
mental results. When the threshold was set in the range 2575
percent of the PDF peak locations, the results did not produce any
significant variations in the flow regime transitions. For ease of
presentation, we use the words bubble and void inter-
changeably in this paper, while recognizing that the voids in the
high-velocity regimes are transitory in nature, not discrete as may
be implied by the term bubble.
For n bubbles passing the lower element of a two-element
probe in time t tot , the bubble frequency is
With t i called the gas burst transit time defined as the time
taken by a bubble to pass the probe i.e., t 3 t 1 or t 4 t 2 in Fig.
2, the local gas holdup is then
n
1
g t .
t tot i1 i
(2)
1.5
f U (5)
d vs g
where d vs is the Sauter mean bubble diameter. The linear relation-
ship between f and U g in Fig. 4 then implies that d vs was inde-
pendent of both U g and U l with d vs3 mm. As shown in Fig. 7
below, this is quite consistent with the chord length distributions
for the dispersed bubble flow regime, the regime corresponding to
most points in Fig. 4, and the dispersed bubbles are of the same
order of size and again are greatly dependent on U g at least.
Evidently the bubble size in these flow regimes, at least for the
conditions and position of measurement, is controlled by the dis-
tribution and/or turbulence.
In the slug flow regime, one can observe bullet-shaped Taylor
bubbles and small bubbles in the liquid plugs separating them. In
the churn flow regime, the bullet-shaped bubbles become narrow
and their shapes are distorted. Small bubbles in the liquid plugs
coalesce and generate new bullet-shaped bubbles. The overall
bubble frequency then increases with the gas velocity in the slug
flow regime and decreases with the gas velocity in churn flow.
This difference in trends was used to determine the transition from
slug to churn flow and is shown in Fig. 5.
Bubble Chord Length and its Distribution. Figure 6 pre-
sents experimental results for the average bubble chord length as a
function of the superficial gas and liquid velocities. The average
bubble chord length increases with increasing gas velocity and
decreases with increasing liquid velocity. As the liquid velocity is
increased, a gradual transition takes place between discrete and
dispersed bubble flow.
Some typical distributions of bubble chord length in the dis-
crete and the dispersed bubble flow regimes are presented in Fig.
7. The four left-hand plots are for the discrete bubble flow regime
at U 1 0.0184 m/s, while the four right-hand plots correspond to
the dispersed bubble flow regime at U 1 0.155 m/s. The standard
deviation of the bubble chord length for each operating condition
is also given in the figure. The peak values of the PDF curves
Fig. 7 Probability density distribution of bubble chord length
appear at an average bubble chord length of approximately 5 mm in discrete and dispersed bubble flow regimes for airwater
for the discrete bubble flow and 2.5 mm for the dispersed bubble system. Uncertainty estimate in measurement of U g 2 per-
flow. The standard deviation of the bubble chord length distribu- cent; uncertainty estimate in measurement of U l 1 percent;
tion increases with the gas velocity in both flow regimes. How- uncertainty estimate in measurement of bubble chord length
ever, the standard deviation of the bubble chord length distribu- 10 percent.
n n
bvs
i1
bi
3
i1
bi
2
(6)
since this average gives added weight to large bubbles 28. Fig-
ure 8 plots the Sauter mean bubble chord length and the average
bubble chord length against the superficial gas velocity. The Sau-
ter mean bubble chord length is always greater than the arithmetic
average bubble chord length at the same gas velocity. The average
bubble chord length is always less than the column diameter in the
slug and the churn flow regimes due to the large number of small
bubbles in the system. Both the Sauter mean bubble chord length
and the average bubble chord length increase only slightly with
U g in the slug flow regime which is defined as starting when the
Sauter mean b first exceeds D. The increase is enhanced in
churn flow. Typical bubble chord length distributions in the slug
and churn flow regimes are presented in Fig. 9. Note that this
figure provides an indication of the entire bubble population. For
example in the slug flow regime, both the Taylor bubbles, prima-
rily responsible for the overall hydrodynamics, and the small
bubbles, primarily responsible for mass transfer between the
phases, are portrayed.
Fig. 8 Bubble chord length in coalesced bubble, slug and
churn flow regimes for airwater system with Z 0.65 m and
It is seen that the average bubble chord length and the standard
D 82.6 mm. Uncertainty estimate in measurement of U g 2 deviation for slug flow left-hand side of Fig. 9 under different
percent; uncertainty estimate in measurement of U l 1 per- operating conditions vary from 21 to 31 mm and from 35 to 52
cent; uncertainty estimate in measurement of bubble chord mm, respectively, while the peaks of the PDF of the bubble chord
length10 percent. length appear at a bubble chord length of 67 mm. This indicates
Fig. 11 Relationship between bubble travel length and aver-
3 2 age bubble chord length in the slug and churn flow regimes for
g f d Ub d . (7) airwater system at Z 0.65 m, D 82.6 mm, and U g 0.002 6
6 vs 4 vs
ms. Uncertainty estimate in measurement of U g 2 percent;
Rearrangement of Eq. 7 yields uncertainty estimate in measurement of U l 1 percent; un-
certainty estimate in measurement of bubble velocity and
g 2 bubble chord length10 percent.
U b d vs . (8)
f 3
The left-hand side of this equation, g U b / f , which we call the
bubble travel length, is plotted against the average bubble chord Three distinctive regions corresponding to different flow regimes
length in Fig. 11 for the discrete and the dispersed bubble flow determined by the methods proposed by Zhang et al. 28 can be
regimes. A nonlinear relationship between the bubble travel found in this figure. At lower average bubble chord length, corre-
length and the average bubble chord length is observed. This sponding to the discrete and dispersed bubble flow regimes, the
could be due to changing bubble shape with increasing bubble relationship between the bubble travel length, and the average
diameter and to other deviations from the assumption of uniform bubble chord length can be correlated by Eq. 9. At intermediate
spherical bubbles. The relationship between the bubble travel average bubble chord length, corresponding to the slug and churn
length and the average bubble chord length for the discrete and flow regimes, the relationship between the bubble travel length
the dispersed bubble flow regimes can be correlated by and the average bubble chord length can be expressed by another
empirical correlation
g
U 0.007 30 log b 0.0211 SI units . (9) g
f b
U 0.1312 log b 0.2276 SI units . (10)
Figure 11 presents all the experimental results for the bubble f b
travel length with respect to the average bubble chord length. It is also seen in Fig. 11 that at high average bubble chord
length, corresponding to the bridging and the annular flow re-
gimes, the experimental data for the bubble travel length are sig-
nificantly greater than predicted by Eq. 10. The relationship be-
tween the bubble travel length and the average bubble chord
length can also be used as an alternative method to determine the
flow regimes in gasliquid cocurrent upward systems. By measur-
ing the bubble/void characteristics with a two-element conductiv-
ity probe, if the measured bubble velocity, gas holdup, bubble
frequency, and average bubble chord length satisfy Eq. 9, then
the flow pattern corresponds to discrete or dispersed bubble flow.
If, on the other hand, the measured bubble characteristics satisfy
Eq. 10, then we have slug or churn flow. If the bubble travel
length is significantly greater than predicted by either Eq. 9 or
Eq. 10, then the flow pattern is either bridging or annular flow.
The difference between the slug and the churn flow regimes can
be seen from a plot of the average bubble velocity versus the
average bubble chord length, as shown in Fig. 12. The dashed line
in the figure corresponds to the flow regime boundary between
these two regimes in Fig. 3. The average bubble velocity increases
sharply as the average bubble chord length varies from approxi-
mately 0.02 to 0.03 m in the slug flow regime. In the slug flow
regime, the average bubble velocity is not only dependent on the
Fig. 10 Average bubble velocity in discrete and dispersed
flow at different superficial liquid velocities for airwater sys-
average bubble chord length, but also on the superficial gas ve-
tem at Z 0.65 m. Uncertainty estimate in measurement of U g locity. As discussed above, the average bubble chord length does
2 percent; uncertainty estimate in measurement of U l not change significantly as the superficial gas velocity varies from
1 percent; uncertainty estimate in measurement of bubble approximately 0.05 to 1 m/s, due to the large number of small
velocity and bubble chord length10 percent. bubbles entrained in slug wakes in the slug flow regime. Hence, a